Robust Ferromagnetism of Chromium Nanoparticles Formed in Superfluid Helium.
نویسندگان
چکیده
Chromium nanoparticles are formed using superfluid helium droplets as the nanoreactors, which are strongly ferromagnetic. The transition from antiferromagentism to ferromagnetism is attributed to atomic-scale disorder in chromium nanoparticles, leading to abundant unbalanced surface spins. Theoretical modeling confirms a frustrated aggregation process in superfluid helium due to the antiferromagnetic nature of chromium.
منابع مشابه
Nanoparticle dispersion in superfluid helium.
Cryogenic fluid flows including liquid nitrogen and superfluid helium are a rich environment for novel scientific discovery. Flows can be measured optically and dynamically when faithful tracer particles are dispersed in the liquid. We present a reliable technique for dispersing commercially available fluorescent nanoparticles into cryogenic fluids using ultrasound. Five types of fluorescent na...
متن کاملDynamics of low-energy helium vapor pulses.
We report results of experiments in which pulses of helium vapor are produced by a current pulse in a chromium film covered with superfluid helium at around 0.3 K. The pulses were detected by a titanium bolometer operating at 0.47 K. The shape of the detected signal is a strong function of the power of the initiating current pulse. For low powers the signal from a single current pulse also cont...
متن کاملSolvation and Spectral Line Shifts of Chromium Atoms in Helium Droplets Based on a Density Functional Theory Approach
The interaction of an electronically excited, single chromium (Cr) atom with superfluid helium nanodroplets of various size (10 to 2000 helium (He) atoms) is studied with helium density functional theory. Solvation energies and pseudo-diatomic potential energy surfaces are determined for Cr in its ground state as well as in the y(7)P, a(5)S, and y(5)P excited states. The necessary Cr-He pair po...
متن کاملVortex-induced aggregation in superfluid helium droplets.
The formation of Ag nanoparticles by the addition of Ag atoms to helium droplets has been investigated. The resulting nanoparticles were then imaged by transmission electron microscopy after being deposited on a thin solid surface. In large helium droplets chains of Ag nanorods were observed similar to recently reported track-like deposits [Gomez et al., Phys. Rev. Lett., 2012, 108, 155302]. Ho...
متن کاملCritical flow and dissipation in a quasi–one-dimensional superfluid
In one of the most celebrated examples of the theory of universal critical phenomena, the phase transition to the superfluid state of (4)He belongs to the same three-dimensional (3D) O(2) universality class as the onset of ferromagnetism in a lattice of classical spins with XY symmetry. Below the transition, the superfluid density ρs and superfluid velocity v s increase as a power law of temper...
متن کاملذخیره در منابع من
با ذخیره ی این منبع در منابع من، دسترسی به آن را برای استفاده های بعدی آسان تر کنید
عنوان ژورنال:
- Advanced materials
دوره 29 1 شماره
صفحات -
تاریخ انتشار 2017